CCS and Power Systems
Crosscutting Research - University Training and Research
Computational Fluid Dynamic Simulations of a Regenerative Process for Carbon Dioxide Capture in Advanced Gasification Based Power Systems
Performer: Illinois Institute of Technology
Project No: FE0003997
A CO2 sorbent regeneration process will be experimentally and computationally studied. The experimental effort will include obtaining the data necessary to determine the intrinsic reaction rates and diffusivity parameters for the CO2 absorption/regeneration and the WGS reactions. A multi-phase Computational Fluid Dynamics (CFD) model is proposed which includes a population balance equation governing the particle porosity distribution (PPD) evolution. The CFD/Population Balance Equation (PBE) model will be numerically solved and simulations of the regenerative carbon dioxide removal process will be performed; the Finite size domain Complete set of trial functions Method Of Moments (FCMOM) numerical technique will be used and developed to solve the PBE. The simulation results will be used to determine the optimum reactor configuration/geometry and the operating conditions for the CO2 removal and hydrogen production.